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An accurate bilayer thickness within the laminate can be readily determined from X-ray re ectivity (XRR) measurements, which also provide con rmation of the abrupt interfaces (<02 nm by XRR) that are visually evident in Fig 412 Although we have not fully characterized the physical properties of the laminates, they do offer unique opportunities for development of highly structured dielectrics For tuning purposes, individual lm thickness can already be varied in a controllable manner from 3 to several hundred nanometers In addition, the lm stack can be deposited with variable levels of hydration, providing explicit control over lm interdiffusion For example, high-order dehydrated stacks exhibiting stability to high temperatures can be produced by dehydrating individual lms during each deposition step.

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(b) Comparison between all SNRs and INRs of 21.0 dB, and all at 21.0 dB except the interferer at 80' which has an INR of 9.0 dB.

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143 DEPOSITION APPROACHES Coupled intimately to the development of the precursors and processing is the development of suitable deposition technologies capable of meeting the complex needs of uniformity, thickness, resolution, and rate For some applications, such as semiconductors, the focus may be on large-area uniformity, whereas for other applications, such as non linear optics, thickness control may be key As a speci c example, contact printing for silicon photovoltaics requires high-resolution lines (<50 m wide) on 6-inch wafers at a processing rate of one wafer per second To achieve these deposition goals, we have seen a variety of techniques in this book, including dip coating, chemical bath deposition, electrodeposition, spray deposition, and printing approaches, such as ink jet, gravure, and offset (eg, see s 6 8 and 12) A next generation of techniques includes nano-pen deposition and stamping approaches.

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Alternatively, stacks can be initially deposited at low temperatures with retention of water and then subsequently heated at higher temperatures to promote intermixing, providing pathways to the formation of selected compositions or compositionally graded lms; in addition, differential crystallization of individual lms can be harnessed to fabricate crystalline high-dielectric lms interleaved with amorphous low-leakage lms Here, the unique precursor chemistries and condensation processes are providing an entirely new, cost-effective bench-top approach to the deposition, study, and development of oxide lms with capabilities currently unknown with conventional vapor-based methodologies..

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23 28 Each of these deposition techniques has pros and cons The best deposition approach in the long run will be application speci c and depend critically on such issues as value added versus cost and resolution and throughput Spray deposition, chemical bath deposition, and dip coating will likely be most useful in areas where uniform large-area coverage is needed dip coating and chemical bath deposition preferably for thin lms and spray deposition for thicker lms Ink-jet printing will have application in elds where patterning 2D or 3D-structures is needed, although it can also be used for deposition of thin homogenous lms Electrodeposition can be used for deposition of thin lms and to thicken patterned materials deposited by ink-jet printing Finally dip pen and stamping approaching can move solution deposition into the nanoscale regime.

The TIP s three different modes are shown in Figure 18-22. To close the TIP (which really just returns it to its near-hidden location on the side of the screen), just tap the Close window button. If you want to return the TIP to its previous behavior of docking at the top or bottom of the screen, click the Tools button and choose the appropriate option: Docking and then Float, Dock at top of screen, or Dock at bottom of screen. Float is the default behavior.

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